Ivan Scheblykin
Professor
Time-resolved photoluminescence studies of single interface wurtzite/zincblende heterostructured InP nanowires
Author
Summary, in English
The interface between wurtzite and zinc blende InP has been identified as type-II, where electrons gather on the zinc blende side and holes on the wurtzite side of the interface. The photoluminescence resulting from recombination across the interface is expected to be long-lived and to exhibit non-exponential decay of emission intensity after pulsed excitation. We verify this prediction using time-resolved photoluminescence spectroscopy on nanowires containing a single heterostructure between a single segment of wurtzite and zinc blende. We find that a significant intensity of type-II emission remains even more than 30 ns after excitation. The decay of the emission intensity is also non-exponential and considerably longer than the exponential decay of the wurtzite InP segment (260 ps). Our results are consistent with the expected photoluminescence characteristics of a type-II interface between the two polytypes. We also find that the lifetime becomes shorter if we create an electron gas at the interface by n-type doping the entire wurtzite segment of the nanowire. This is expected since there are many electrons that a given hole can recombine with, in contrast to the undoped case.
Department/s
- NanoLund: Centre for Nanoscience
- Solid State Physics
- Chemical Physics
- Centre for Analysis and Synthesis
Publishing year
2022-03-14
Language
English
Publication/Series
Applied Physics Letters
Volume
120
Issue
11
Links
Document type
Journal article
Publisher
American Institute of Physics (AIP)
Topic
- Condensed Matter Physics (including Material Physics, Nano Physics)
- Nano-technology
Status
Published
ISBN/ISSN/Other
- ISSN: 0003-6951